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The Plimpton Family Papers is primarily comprised of correspondence, personal and professional documents, writings and photographs generated by or for George Arthur Plimpton and Frances Taylor Pearsons Plimpton, their son, Francis T.P. Plimpton, and his wife Pauline Ames Plimpton. Also included are documents and photographs produced by or for other Plimpton, Pearsons and Ames family members, from seventeenth century ancestors to late-twentieth century descendants.

The Historical Photo Collection contains images of persons, events, and activities associated with Columbia College (1754-1896) and Columbia University (1896-).

This collection contains records documenting Columbia University's activities slightly prior to, during and immediately following World War I. The collection consists of mostly correspondence, but also includes newspaper clippings, pamphlets, various publications, reports, photographs, service record cards, and numerous lists of Columbia men and women who served during the war.

The Historical Subject Files Collection documents Columbia University history and related topics from 1754 to the present. The collection includes articles, booklets, clippings, correspondence, memoranda, non-photographic images, notes, pamphlets, posters, press releases, programs and reports.

The office files of the University Librarian's Office of Columbia University Libraries, 1889-1948, are composed is composed chiefly of correspondence sent and received between Columbia University Librarians, library staff, Columbia University administrators, and outside individuals and organizations, as well as related reports, budgets, as well as related reports, budgets, and administrative material concerning the history of the library.

A significant collection of Rockwell Kent's correspondence; drawings and sketches; watercolors; lithographs; proofs; manuscripts; and architectural drawings. There are also lithographs and woodblock prints by Kent's students and admirers.

The George A. Plimpton Papers consist largely of personal and professional correspondence, financial and real estate records, personal diaries and albums, writings, and lectures produced by or for George Arthur Plimpton. But the Papers also contains not only the correspondence and records of Plimpton's colleagues at Ginn and Company, the publishing house that Plimpton led for decades, but also correspondence and records relating to the dozens of other institutions and organizations that Plimpton helped lead. In addition to extensive correspondence relating to Plimpton's collecting of rare books, manuscripts, and historical artifacts, the Papers also contain such diverse items as autographs of presidents, handwriting specimens, studies of medieval manuscripts, and documents relating to the American slave trade.