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Correspondence, notes, articles, reports, and speeches of Gildersleeve, including materials relating to the United Nations Conference in San Francisco, 1945, the Dumbarton Oaks Conference, the International Federation of University Women, the American Association of University Women, the American Council on Education, and the Near East College Association. The most note-worthy item in the collection is a letter from President Franklin D. Roosevelt, appointing Dean Gildersleeve to serve as a member of the U.S. Delegation to the Charter Conference of the United Nations. The collection also contains some material relating to Barnard College affairs.

Correspondence, manuscripts, notes, memoranda, notebooks, notecards, proofs, photographs, microfilms, and printed materials. The Papers include the manuscript research materials and correspondence for each of his books except his biography of Theodore Dreiser. Among the correspondents are William Benton, Bruce Catton, Carey McWilliams, Mrs. Fremont Older (Cora Miranda Baggerly Older), and Thornton Wilder.