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The papers include correspondence, subject files, photographs, and printed materials. The majority of the collection concerns the mission of the American Red Cross to Russia in 1917-1918; Thacher served as a secretary of the mission. There are letters and telegrams by W.B. Thompson and Raymond Robins, records of supplies, shipments, and distribution reports and over 600 photographs from Russia, China, and Romania. There is substantial correspondence from 1918-1919 concerning Russia, including letters by Louis Brandeis, Felix Frankfurter, and Lillian Wald. A substantial part of the collection concerns Russian war relief in 1941-1942, an area in which Thacher was active. Printed materials include a pamphlet and an article on Russia prepared by Thacher after his return from that country in early 1918.

Correspondence, documents and manuscripts from late seventeenth and eighteenth century France, especially from the French Revolution, collected by Sam Schaefler. Authors include J.B. Colbert Torcy and the Duchesse Du Lude. Many of the items from the French Revolution represent the work of the Committee of Public Safety and the Committee of General Security. French Revolutionary leaders represented in the collection include François-Antoine Boissy D'Anglas, Jean-Baptiste-Noel Bouchotte, Pierre Joseph Cambon, Lazare Carnot, Jean-Marie Collot D'Herbois, l'Abbʹe de Fauchet, Philippe-Antoine Merlin de Douai, Jean Victor Moreau. C.A. Prieur-Duvernois, and Antoine Joseph Santerre. In addition, the collection includes a letter from the Danish physicist Hans Christian Oersted to Sir John Herschel, a letter by the French poet Romain Rolland, a document of the Philadelphia Artists' Fund Society of 1846 with signatures of its officers, and an autograph letter and a photograph of Henry Wadsworth Longfellow.