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Letters written to Gay from political and literary contemporaries such as Horace Greeley, Charles Sumner, and William Bryant; reports in letter form from his reporters at the front during the Civil War; and personal correspondence including many letters from his wife, Elizabeth Neall Gay. Letters written to Mrs. Gay from family friends and business associates including many from her husband. Correspondence of other members of the Gay family including Walter Gay, Sarah Gay, and Allan Gay. Diaries, notebooks, and journals of Sydney Howard Gay.

Correspondence of Nikola Tesla and Robert Underwood Johnson include letters of Tesla to Johnson's wife and daughter, clippings, photographs, and miscellaneous materials. Letters to George Scherff, 1902-1930, and others, manuscripts, printed articles, patents, and brochures. The material is of a technical nature and the letters deal primarily with Tesla's work on transformers, turbines, steam and gas oscillators, compressors, pumps, induction motors, and wireless transmitters. Also, printed materials by and about Tesla, including DR. NIKOLA TESLA BIBLIOGRAPHY (1979) by John T. Ratzlaff and Leland I. Anderson; and published selections from diary entries, correspondence, patents, and patent wrappers by Tesla published by the Tesla Book Company. There is also a videotape cassette "Nikola Tesla the Genius Who Lit the World".

Correspondence and manuscripts of various literary figures, occasionally brought for this library by the Friends of the Columbia University Libraries. Authors include William Harrison Ainsworth, Augustine Birrell, Thomas Campbell, James Fenimore Cooper, Clement Clarke Moore, Carl Sandburg, A. C. Swinburne, Dylan Thomas, Anthony Trollope, and Talcott Williams.