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Papers documenting Longwell's influential career in publishing and journalism. There are files of correspondence with such notables as Sir Winston Churchill, Ernest Hemingway, Thomas Hart Benton, the Duke and Duchess of Windsor, Christopher Morley, and H.L. Mencken as well as artists such as Tom Lea and Peter Hurd. Also, correspondence and memoranda dealing with the Time-Life organization, among them an extensive series of letters from Henry R. Luce and various editors of the magazines.

Correspondence, manuscripts, diaries, drafts, notes, documents, proofs, clippings, printed books, and other related materials. There are typescript drafts, proofs, related correspondence,, and printed copies of each of her books; typescript and tearsheets of her short stories, novelettes, and playscripts; correspondence with readers, agents, and publishers, and files for her promotional work at Time-Life, her newspapare and magazine columns, and her other interests; her daily appointment books; and her financial records. Among the cataloged correspondence are: Roger Nash Baldwin, Moss Hart, Hubert H. Humphrey, Ernest Jones, Clare Boothe and Henry Luce, Thomas Mann, Jo Mielziner, and Dorothy Thompson.

The collection consiste of correspondence, memoranda, reports, bulletins, clippings, photographs, awards, and printed material. The files, arranged by genre and topic and reflect her philanthropic and legislative work in the areas of health, specifically cancer, heart disease, and mental health. Her civic and legislative work is covered in detail, as well as her private interests and activities.

Correspondence, manuscripts, notes, memoranda, notebooks, notecards, proofs, photographs, microfilms, and printed materials. The Papers include the manuscript research materials and correspondence for each of his books except his biography of Theodore Dreiser. Among the correspondents are William Benton, Bruce Catton, Carey McWilliams, Mrs. Fremont Older (Cora Miranda Baggerly Older), and Thornton Wilder.

Correspondence, manuscripts, dispatches, documents, clippings and other printed materials concerning his career as an editor and correspondent for the New York Herald Tribune in Moscow, Berlin and New York, as a staff member of the Institute of Pacific Relations from 1932 to 1934, as deputy director in the Office of War Information overseas branch, 1941-44, as an owner and editor of the New York Star, 1948-49, as an instructor in communications at Sarah Lawrence College, 1950-1951, as a book editor at Simon and Schuster, Publishers, 1951-1970, and as an author and translator.