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The Plimpton Library of 16,000 volumes- a 1936 gift of George A. Plimpton - covers what the collector called "our tools of learning" from the fifteenth to the late nineteenth centuries. The cataloged books are described in the card catalog and in CLIO. There are a good number of uncataloged books, which are classed in Dewey, and findable through a shelflist and an author catalog.

This collection includes hornbooks, battledores, and facsimiles of hornbooks, a few hornbook-adjacent items, and supporting documents. Hornbooks and battledores were used from the 14th through the 19th centuries for the earliest steps of training in literacy: learning to recognize letterforms, and sometimes to read syllables and/or short texts.

Primarily oil portraits of 18th century literary figures. There are also engravings, and pen and ink and pencil sketches. Among the literary figures are portraits of Samuel Butler, Lord Byron, Thomas Carlyle; Colley Cibber; Charles Dickens; John Evelyn; John Foxe; David Garrick; Thomas Gray; Charles Lamb; Sir Thomas More; Sir Walter Raleigh; Samuel Richardson; Richard B. Sheridan; Alfred, Lord Tennyson; William M. Thackeray; and others. There is also a portrait by Blanche Ames of George A. Plimpton. Among the artists represented in the collection are James Maubert, Frederick Sandys, and William Hogarth (attrib.)

Correspondence, minutes of meetings, financial records, publications, notes, subject files, awards, speeches, reports and audiovisual materials document work by the Church Peace Union, its successors Council on Religion in International Affairs and Council on Ethics and International Affairs, and related organizations such as the World Alliance for International Friendship Through the Churches. The first installment of the CCEIA archival materials came to the RBML in 1974, with numerous additions over the years. A major addition in 1982 contained primarily the records of the Board of Directors and their semi-annual meetings, as well as the various programs and institutes of the Council, for the years 1972-1982, along with selected 1930s materials. 1986 addition contains presidential correspondence files, minutes of the Board of Trustees and committees, special projects, programs and conferences files, and the business and editorial files of "Worldview". Correspondents include John Foster Dulles, Jane Addams, Fiorello La Guardia, and Paul Tillich. 1990 and 2000 additions includes files of CCEIA presidents and vice presidents, paper and audiovisual materials on Merrill House Conversation Programs; Educational programs; International Monetary Fund/Lecture series; The Annals Of The Academy Of Political & Social Science; Washington Consultations; Colloquia for the Clergy; Church State Project; Asian Development & The Carribean Initiative; Korea: Year 2000 Project; fundraising files, printed materials and files of the Department of Publications.