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The career, philanthropic, political, and personal aspects of Charles Richard Crane's life were closely intertwined. Among the correspondence of significance in the papers are letters to and from James Francis Abbott, Kathryn Newell Adams, Jane Addams, Edmund Henry Hynman Allenby, Edvard Benes, Boris III, King of Bulgaria, Louis Dembitz Brandeis, Nicholas Murray Butler, Frances F. Cleveland, Grover Cleveland, Archibald Gary Coolidge, Calvin Coolidge, John Dewey, Charles William Elliot, Hamlin Garland, William Rainey Harper, Jean-Jules Jusserand, William Lyon Mackenzie King, Alexander Kuprin, Robert Marion LaFollette, Seth Low, William Gibbs McAdoo, Jan Masaryk, Tomas Masaryk, Pavel Miliukov, John Pierpont Morgan, Alphonse Maria Mucha, Fridtjof Nansen, George Haven Putnam, John Davison Rockefeller Jr., Theodore Roosevelt, Upton Beall Sinclair, William Howard Taft, Lillian D. Wald, Herbert George Wells, Edith B. Wilson, Woodrow Wilson and other.

This collection contains architectural drawings, photographs, business records and reference materials related to the projects and designs of Bertram Grosvenor Goodhue and his successor firm, Mayers, Murray & Philips, primarily in the New York City region. A large portion of the collection consists of personal and professional correspondence to and from Goodhue from the early 1900s until his death in 1926. Relatively few architectural drawings from his professional practice survive.